Challenge: Recent trends have led to the use of multimodal models to learn molecular and linguistic representations, either in separate but coordinated spaces or in a common space.
Approach: They propose a novel atomic-level evaluation method leveraging off-the-shelf Natural Language Inference (NLI) models for use in the unseen chemical domain.
Outcome: The proposed method surpasses state-of-the-art models in the unseen chemical domain while relying on a granularity-based evaluation method.

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A Survey of Large Language Models for Text-Guided Molecular Discovery: From Molecule Generation to Optimization (2026.acl-long)

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Challenge: Large language models (LLMs) are introducing a paradigm shift in molecular discovery by enabling text-guided interaction with chemical spaces through natural language and symbolic notations.
Approach: They analyze the current LLM learning paradigms to tackle four critical evaluation dimensions that have emerged as critical dimensions in recent studies.
Outcome: The proposed models are able to interact with chemical spaces through natural language and symbolic notations, and have emerging extensions to incorporate multi-modal inputs.
Leveraging Large Language Models for NLG Evaluation: Advances and Challenges (2024.emnlp-main)

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Challenge: introducing Large Language Models (LLMs) has opened new avenues for assessing generated content quality, e.g., coherence, creativity, and context relevance.
Approach: They propose a taxonomy for organizing existing LLM-based evaluation metrics and a structured framework to understand and compare them.
Outcome: The proposed taxonomy offers a framework to understand and compare LLM-based evaluation methods.
Enhancing Cross Text-Molecule Learning by Self-Augmentation (2024.findings-acl)

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Challenge: Existing datasets are limited due to the difficulty of collecting precise molecule-description pairs. Existing approaches to enhance large language models include a data augmentation framework and a new dataset called SAPubChem-41.
Approach: They propose a framework that interweaves model fine-tuning and data augmentation to overcome the scarcity of high-quality labeled data.
Outcome: The proposed framework interweaves model fine-tuning and data augmentation to overcome the scarcity of high-quality labeled data.
Improving the OOD Performance of Closed-Source LLMs on NLI Through Strategic Data Selection (2026.findings-eacl)

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Challenge: Existing methods to improve robustness require changing the fine-tuning process or large-scale data augmentation, which are infeasible or cost prohibitive for closed-source models.
Approach: They propose to prioritize more complex examples or replace existing training examples with LLM-generated data to improve performance on OOD NLI datasets.
Outcome: The proposed methods improve performance on difficult OOD datasets while training with synthetic data leads to substantial improvements on easier OOD data.
Lost in Translation: Chemical Language Models and the Misunderstanding of Molecule Structures (2024.findings-emnlp)

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Challenge: chemistry and natural language processing (NLP) have advanced drug discovery.
Approach: They propose a framework for assessment of Chemistry LMs of different natures that relies on augmentations that preserve an underlying chemical.
Outcome: The proposed framework relies on augmentations that preserve an underlying chemical, such as kekulization and cycle replacements.
A synthetic data approach for domain generalization of NLI models (2024.acl-long)

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Challenge: Natural Language Inference (NLI) datasets are important benchmark tasks for LLMs . however, their realistic performance on out-of-distribution/domain data is less well-understood . a T5-small model trained with our data improves around 7% on average compared to the best alternative dataset .
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Outcome: The proposed model can be trained on datasets with high-quality examples with meaningful premises and high accuracy.
Cool-Fusion: Fuse Large Language Models without Training (2025.acl-long)

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Challenge: Cool-Fusion is a simple yet effective approach to combine two or more heterogeneous large language models .
Approach: They propose a method that fuses the knowledge of two or more heterogeneous large language models to leverage complementary strengths.
Outcome: The proposed method increases accuracy from three strong source LLMs on GSM8K by 17.4%.
Feedback to Reasoning: LLM-Assisted Molecular Optimization with Domain Feedback and Historical Reasoning (2026.findings-acl)

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Challenge: Existing methods for molecular optimization do not leverage domain feedback and historical knowledge with reasoning traces and chemical insights.
Approach: They propose a conversational molecular optimization pipeline that enables LLMs to accumulate and retrieve past actions, rationales, and feedback.
Outcome: The proposed framework transforms LLMs from passive text generators into agentic experts that learn both actions and reasoning from experience.
RetroLLM: Empowering Large Language Models to Retrieve Fine-grained Evidence within Generation (2025.acl-long)

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Challenge: Existing methods rely on separate retrievers to fetch top-k text chunks for generating evidence, and they lack joint optimization.
Approach: They propose a framework that integrates retrieval and generation into a single, auto-regressive process, enabling LLMs to directly generate fine-grained evidence from the corpus with constrained decoding.
Outcome: Extensive experiments on five open-domain QA datasets demonstrate the proposed framework’s superior performance across both in-domain and out-of-domain tasks.
Translation between Molecules and Natural Language (2022.emnlp-main)

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Challenge: MolT5 pretrains models on unlabeled natural language text and molecule strings . bringing a new drug to market can cost over a billion dollars and take over ten years .
Approach: They propose a self-supervised learning framework for pretraining models on unlabeled natural language text and molecule strings.
Outcome: The proposed framework pretrains models on unlabeled natural language text and molecule strings, and it generates high quality outputs.

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