Challenge: Recent advances in large language models (LLMs) have shown significant performance, approaching human perception levels.
Approach: They propose an approach that sketches molecular structures for reasoning by explicitly incorporating key structural features into the model.
Outcome: The proposed framework improves molecular understanding through extensive experiments.

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Boosting LLM’s Molecular Structure Elucidation with Knowledge Enhanced Tree Search Reasoning (2025.acl-long)

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Challenge: Molecular structure elucidation involves deducing a molecule’s structure from various types of spectral data, which is crucial in chemical experimental analysis.
Approach: They propose a Knowledge-enhanced reasoning framework for Molecular Structure Elucidation that leverages Monte Carlo Tree Search for test-time scaling as a plugin to extend the LLMs’ coverage of the chemical structure space.
Outcome: The proposed framework significantly improves on both GPT-4o-mini and GPT4o, and a specialized molecule-spectrum scorer improves performance.
Current Advances in LLM Reasoning (2026.acl-tutorials)

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Challenge: This tutorial examines comprehensive evaluation strategies to assess the reasoning abilities of large language models (LLMs) advanced inference time methods and post-training methods that aim to make LLMs think more like humans are discussed in this tutorial.
Approach: This tutorial explores comprehensive evaluation strategies to assess the reasoning abilities of large language models (LLMs) and discusses two types of methods to improve models’ reasoning: advanced inference time methods, structured and self-improvement inference methods, and post-training methods, such as RLHF, DPO, and GRPO.
Outcome: This tutorial examines evaluation strategies to assess the reasoning abilities of large language models and discusses two types of methods to improve models’ reasoning.
MolRAG: Unlocking the Power of Large Language Models for Molecular Property Prediction (2025.acl-long)

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Challenge: Recent LLMs exhibit limited effectiveness on molecular property prediction task due to semantic gap between representations and natural language and lack of domain-specific knowledge.
Approach: They propose a framework that integrates Chain-of-Thought reasoning for molecular property prediction.
Outcome: The proposed framework outperforms pre-trained LLMs on four datasets and matches supervised methods.
A Survey of Large Language Models for Text-Guided Molecular Discovery: From Molecule Generation to Optimization (2026.acl-long)

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Challenge: Large language models (LLMs) are introducing a paradigm shift in molecular discovery by enabling text-guided interaction with chemical spaces through natural language and symbolic notations.
Approach: They analyze the current LLM learning paradigms to tackle four critical evaluation dimensions that have emerged as critical dimensions in recent studies.
Outcome: The proposed models are able to interact with chemical spaces through natural language and symbolic notations, and have emerging extensions to incorporate multi-modal inputs.
Feedback to Reasoning: LLM-Assisted Molecular Optimization with Domain Feedback and Historical Reasoning (2026.findings-acl)

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Challenge: Existing methods for molecular optimization do not leverage domain feedback and historical knowledge with reasoning traces and chemical insights.
Approach: They propose a conversational molecular optimization pipeline that enables LLMs to accumulate and retrieve past actions, rationales, and feedback.
Outcome: The proposed framework transforms LLMs from passive text generators into agentic experts that learn both actions and reasoning from experience.
Improving Chemical Understanding of LLMs via SMILES Parsing (2025.emnlp-main)

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Challenge: Molecular string representations such as SMILES and SELFIES are becoming a standard format for applying large language models (LLMs) however, molecular strings follow complex syntactic rules for encoding molecules, which LLMs struggle to interpret.
Approach: They propose a framework that parses SMILES into clean and deterministic tasks to promote graph-level molecular comprehension.
Outcome: The proposed framework improves structural comprehension and competes with the baseline on the Mol-Instructions benchmark.
Towards Reasoning in Large Language Models: A Survey (2023.findings-acl)

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Challenge: Reasoning is a fundamental aspect of human intelligence that plays a crucial role in many intellectual activities.
Approach: They propose to improve LLMs' ability to elicit reasoning by providing exemplars or prompts to model reasoning.
Outcome: This paper provides a comprehensive overview of the state of knowledge on reasoning in large language models.
Exploring the Role of Reasoning Structures for Constructing Proofs in Multi-Step Natural Language Reasoning with Large Language Models (2024.emnlp-main)

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Challenge: Large language models (LLMs) are essential for performing complex multi-step reasoning tasks, such as multi-hop reasoning tasks.
Approach: They propose to use large language models to derive structured intermediate proof steps to improve their performance by using examples.
Outcome: The proposed models can derive correct proof steps with in-context learning.
SR-LLM: Rethinking the Structured Representation in Large Language Model (2025.acl-long)

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Challenge: Structured representations have long been pivotal in computational linguistics, but their role remains ambiguous in the Large Language Models (LLMs) era.
Approach: They propose a framework that integrates structured representations into LLMs from training-free and training-dependent perspectives.
Outcome: The proposed framework integrates structured representations through natural language descriptions in LLM prompts while augmenting the model’s inference capability through fine-tuning on linguistically described structured representation.
Advancing Reasoning with Off-the-Shelf LLMs: A Semantic Structure Perspective (2025.findings-emnlp)

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Challenge: Existing reasoning models suffer from hallucinations and unfaithfulness, whereas general LLMs perform suboptimal on complex tasks.
Approach: They propose a structure analysis method that helps LLMs better understand the question structure and guide the problem-solving process.
Outcome: The proposed method improves zero-shot performance on knowledge-intensive and mathematical tasks while demonstrating strong robustness against corrupted reasoning paths.

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